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In article number 1906432, Dan‐Hong Wang, Xian‐He Bu, and co‐workers present a novel design strategy aiming to form heteropoly blues confined in defected Zr‐metal–organic framework (MOF), which can expose more unsaturated metal sites to promote the catalytic activity by adding thiourea. Moreover, 1‐butyl 3‐methyl imidazolium phosphomolybdate blues are also confined in Zr‐MOF to obtain higher oxidative...
The Keggin‐type polyoxometalates (POMs) are effective catalysts for oxidative desulfurization (ODS) and confining these POMs in metal–organic frameworks (MOFs) is a promising strategy to improve their performances. Herein, postsynthetic modification of POMs confined in MOFs by adding thiourea creates more unsaturated metal sites as defects, promoting ODS catalytic activity. Additional modification...
Electronic structure of active sites plays a crucial role in redox catalysts. Herein, graphitic carbon nitride (g-C3N4) decorated with metallic MoO2 heterojunction nanocomposites were successfully synthesized through a facile calcination route. XPS, UPS, UV–vis and PL spectra results suggest electron transfer from the conduction band (CB) of g-C3N4 to unfilled π* band of metallic MoO2 in the metal-semiconductor...
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