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Reported here is the synthesis, solid‐state characterization, and redox properties of new triangular, threefold symmetric, viologen‐containing macrocycles. Cyclotris(paraquat‐p‐phenylene) (CTPQT6+) and cyclotris(paraquat‐p‐1,4‐dimethoxyphenylene) (MCTPQT6+) were prepared and their X‐ray single‐crystal (super)structures reveal intricate three‐dimensional packing. MCTPQT6+ results in nanometer‐sized...
Metall‐organische Gerüste (MOFs) sind Hybridmaterialien, die anhaltendes Interesse auf sich ziehen – nicht zuletzt wegen vielfältiger möglicher Anwendungen, von der Gastrennung über die Katalyse bis hin zum Sammeln von Licht. Allerdings ist die De‐novo‐Synthese von MOFs mit gewünschten Eigenschaften nicht immer einfach: unerwünschte Topologien können entstehen, die Löslichkeit von Vorstufen kann zu...
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