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Polyoxometalate‐like behavior of actinyl‐peroxide anions in aqueous alkaline media has been recently unveiled in the form of more than 20 reported crystal structures of clusters, each with 20–60 uranyl polyhedra composing capsule‐like topologies. There is now opportunity to fully develop this new polyoxometalate (POM) family to include redox behavior, non‐aqueous chemistry, complex materials from...
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