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The near-infrared (700-1900 nm) magnetic circular dichroism (MCD) spectra of a horse-heart metmyoglobin-imidazole complex have been measured as a function of pD between 9.1 and 12.2 at room temperature. Two low-spin ferric haem complexes with MCD peaks at 1600 and 1350 nm, respectively, interconvert with an apparent pK a of just above 11.0. Since this process has been identified with the deprotonation...
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