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Resonance Raman (RR) spectra of free‐base meso‐tetra(p‐hydroxyphenyl)porphine(THPP) were obtained with 397.9, 416 and 514 nm excitation wavelengths, and density functional calculations were carried out to help the elucidation of the photorelaxation dynamics of Soret (Bx and By bands) electronic transitions and the RR spectra of THPP. The RR spectrum indicates that the Franck–Condon (FC) region photorelaxation...
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