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Layer flexibility in two‐dimensional coordination polymers (2D‐CPs) contributes to several functional materials as it results in anisotropic structural response to external stimuli. Chemical modification is a common technique for modifying layer structures. This study demonstrates that crystal morphology of a cyanide‐bridged 2D‐CP of type [Mn(salen)]2[ReN(CN)4] (1) consisting of flexible undulating...
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