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A host–guest molecular recognition is reported between cucurbit[7]uril and butyrylcholine with the driving forces of hydrophobic and charge-dipole interactions. On the basis of this recognition, an enzyme- and photo-responsive supramolecular amphiphile is fabricated, which self-assembles into vesicles in aqueous solution. The assembly and disassembly of vesicles are successfully employed in stimuli-triggered...
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