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A new hybrid local and charge transfer (HLCT) molecule 2TPA‐PPI is obtained for constructing the high‐performance organic light‐emitting diodes (OLEDs) in this work. 2TPA‐PPI possesses the sufficient emission/charge‐transporting properties, thus it is used as a neat emitter achieving an efficient deep‐blue OLED with very high external quantum efficiency (EQE) up to 10.7%, as well as a multi‐functional...
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