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The synthesis of large‐scale 2D conductive metal‐organic framework films with tunable thickness is highly desirable but challenging. In this study, an Interface Confinement Self‐Assembly Pulling (ICSP) method for in situ synthesis of 4‐in. Ni‐BHT film on the substrate surface is developed. By modulating the thickness of the confined space, the thickness of Ni‐BHT films could be easily varied from...
Wearable electronics are attracting increasing interest due to the emerging Internet of Things (IoT). Compared to their inorganic counterparts, stretchable organic semiconductors (SOSs) are promising candidates for wearable electronics due to their excellent properties, including light weight, stretchability, dissolubility, compatibility with flexible substrates, easy tuning of electrical properties,...
Adjusting the local coordination environment of single‐atom electrocatalysts is a viable way to improve catalytic performance. The diversity of coordination geometric structures is limited to the traditional in‐plane configuration, with only a little consideration paid to out‐of‐plane configurations due to the lack of suitable carriers and fabrication methods. This study reports out‐of‐plane coordination...
Bifunctional Catalysts
In article number 2201974, Yunqi Liu, Xuan Yang, Xiang Feng, Yuan Pan, and co‐workers propose an encapsulation‐adsorption‐pyrolysis strategy for constructing Co‐Te diatomic sites with special CoN3C1‐TeN1C3 coordination structure anchored in N‐doped carbon, as efficient bifunctional catalysts for synergistic electrocatalytic hydrogen evolution and oxygen reduction. This work...
A encapsulation–adsorption–pyrolysis strategy for the construction of atomically dispersed Co‐Te diatomic sites (DASs) that are anchored in N‐doped carbon is reported as an efficient bifunctional catalyst for electrocatalytic hydrogen evolution reaction (HER) and oxygen reduction reaction (ORR). The as‐constructed catalyst shows the stable CoN3C1‐TeN1C3 coordination structure before and after HER...
Artificial intelligence vision systems (AIVSs) with information sensing, processing, and storage functions are increasingly gaining attention in the science and technology community. Although synapse phototransistor (SPT) is one of the essential components in AIVSs, solution‐processed large‐area photonic synapses that can detect and recognize multi‐wavelength light are highly desirable. One of the...
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