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The dramatic increase in anthropogenic carbon dioxide emissions in recent decades has forced us to look for alternative carbon-neutral processes for the production of energy vectors and commodity chemicals. Photo- and electrochemical reduction of CO2 are appealing strategies for the storage of sustainable and intermittent energies in the form of chemical bonds of synthetic fuels and value-added molecules...
In this account the concept of using formic acid as a hydrogen storage material is presented. Catalytic reduction of carbon dioxide and heterogeneously catalyzed decomposition of formic acid to hydrogen and carbon dioxide are briefly discussed. In the main part the historic development and recent examples of homogeneously catalyzed hydrogen generation from formic acid are covered in detail.
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