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We present the synthesis of two sets of spiro‐connected azaacene dimers. Their geometry and electronic coupling are critically determined by a secondary linker, i. e., an etheno‐ and an ethano‐bridge. The core fragment of the etheno‐bridged dimer corresponds to a conformationally locked cis‐stilbene. Optoelectronic properties, single crystal X‐ray structures and stability with respect to oxidation...
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