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A solvent-free α-alkylation of acetone with butanol and ethanol was conducted using a mixture of Pd/C and CaO as heterogeneous catalysts. After reaction at 180°C for 20h, alkylated products, including C5-C11 ketones and alcohols, were obtained with a total yield of 78.1%. After this α-alkylation, consecutive hydrodeoxygenation at 270°C for 20h under H2 at 500 psig yielded 74.7% C5–C11 alkanes based...
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