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Four 2,2′‐dipyridylamino‐s‐triazine‐substituted ligands, each of which incorporate different aromatic substituents (phenoxo, 4‐CN‐phenoxo and benzylamino) with different degrees of bulk and flexibility, have been formed and incorporated into a number of mononuclear FeII complexes of type trans‐[FeII(L)2(NCX)2]·solvent (in which X = S, Se and BH3). These ligands were designed to promote π–π stacking...
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