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Within this work we have investigated spiro‐based tetrathiafulvalenes (TTFs) obtained as mixtures of stereoisomers from racemic spiro[5.5]undeca‐1,8‐dien‐3‐one. Compared to previously described spiro‐TTFs, enantiomeric and diastereoisomeric forms have been here separated by chiral HPLC and fully characterized both experimentally and theoretically. The two types of spiro‐based chiral derivatives contain...
Manipulation of long‐range order in 2D van der Waals (vdW) magnetic materials (e.g., CrI3, CrSiTe3 ,etc.), exfoliated in few‐atomic layer, can be achieved via application of electric field, mechanical‐constraint, interface engineering, or even by chemical substitution/doping. Usually, active surface oxidation due to the exposure in the ambient condition and hydrolysis in the presence of water/moisture...