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We report a study of the 203 Tl and 205 Tl Nuclear Magnetic Resonance of the ternary semiconductor TlTaS 3 that shows a chain structure. Our measurements show noticeable intra-chain (Tl-Tl) and inter-chain (Tl-Ta) indirect nuclear spin-spin interactions. These couplings result from the overlap of the Tl and Ta electron wave functions across the intervening...
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