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Pd‐NO2‐UiO‐66 for DMC Catalysis
In article number 2208238, Ye‐Yan Qin, Yuan‐Gen Yao, and co‐workers first introduce acidity/alkalinity functionalized metal–organic frameworks (MOFs) into dimethyl carbonate (DMC) catalysis, and the Lewis acidic Pd‐NO2‐UiO‐66 exhibits excellent catalytic behavior. In addition to affecting the interaction of Pd(II) and support, the ‐NO2 group has a dominant role in the...
The acid–base properties of supports have an enormous impact on catalytic reactions to regulate the selectivity and activity of supported catalysts. Herein, a train of Pd‐X‐UiO‐66 (X = NO2, NH2, and CH3) catalysts with different acidity/alkalinity functional groups and encapsulated Pd(II) species is first developed, whose activities in dimethyl carbonate (DMC) catalysis are then investigated in...
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