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High‐voltage lithium metal batteries (LMBs) are capable to achieve the increasing energy density. However, their cycling life is seriously affected by unstable electrolyte/electrode interfaces and capacity instability at high voltage. Herein, a hydrofluoric acid (HF)‐removable additive is proposed to optimize electrode electrolyte interphases for addressing the above issues. N, N‐dimethyl‐4‐(4,4,5,5‐tetramethyl‐1,3,2‐dioxaborolan‐2‐yl)...
Solid electrolyte interphase (SEI) and cathode electrolyte interphase (CEI) with optimized components and structures are considered to be crucial for lithium‐ion batteries. Here, gradient lithium oxysulfide (Li2SOx, x = 0, 3, 4)/uniform lithium fluoride (LiF)‐type SEI is designed in situ by using hexafluoroisopropyl trifluoromethanesulfonate (HFPTf) as electrolyte additive. HFPTf is more likely to...
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