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Electrochemical CO2 Reduction
In article number 2300801, Huan Wang and co‐workers report a graphene–supported Fe–N4O–C nanoplates electrocatalyst that drives a rechargeable Zn–CO2 battery with energy supply and highly efficient conversion of CO2 into CO, an important one‐carbon building block for the synthesis of long‐chain compounds.
Electrochemical carbon dioxide (CO2) reduction into value‐added products holds great promise in moving toward carbon neutrality but remains a grand challenge due to lack of efficient electrocatalysts. Herein, the nucleophilic substitution reaction is elaborately harnessed to synthesize carbon nanoplates with a FeN4O configuration anchored onto graphene substrate (FeN4OC/Gr) through covalent linkages...