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The BN analogue of ortho‐benzyne, 1,2‐azaborine, is generated by flash vacuum pyrolysis, trapped under cryogenic conditions, and studied by direct spectroscopic techniques. The parent BN aryne spontaneously binds N2 and CO2, thus demonstrating its highly reactive nature. The interaction with N2 is photochemically reversible. The CO2 adduct of 1,2‐azaborine is a cyclic carbamate which undergoes photocleavage,...
Isoliertes Produkt: Die Photoisomerisierung von 1,2‐Dihydro‐1,2‐azaborin in Neon‐, Argon‐ oder Xenonmatrices bei 4 K mit UV‐Licht (253.7 nm) im Rahmen einer Matrixisolationsstudie liefert die Dewar‐Form als einziges Photoprodukt, im Einklang mit den berechneten Schwingungsspektren möglicher Isomere des 1,2‐Dihydro‐1,2‐azaborins.
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