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Free energy relationship (FER) studies to correlate steric parameters with the enantiocatalytic performance of bifunctional tertiary‐amine hydrogen‐bonding catalysts, including (S,S)‐cyclohexane‐1,2‐diamine‐derived thioureas, Cinchona alkaloid derived thioureas, and (S,S)‐cyclohexane‐1,2‐diamine‐derived squaramides, in Michael reactions revealed that the reactions are much favored by catalysts with...
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