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We report Seebeck coefficients of electrochemical cells with molten carbonate mixtures as electrolytes and carbon dioxide|oxygen electrodes. The system is relevant for use of waste heat and off-gases with concentration of carbon dioxide different from air, as for example in the metallurgical industry. The coefficient is −1.25mVK−1 for a nearly equimolar mixture of lithium and sodium carbonate with...
The Seebeck coefficient is reported for thermoelectric cells with gas electrodes and a molten electrolyte of one salt, lithium carbonate, at an average temperature of 750°C. We show that the coefficient, which is 0.88mVK−1, can be further increased by adding an inorganic oxide powder to the electrolyte. We interpret the measurements using the theory of irreversible thermodynamics and find that the...
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