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Why would the pressure of hydrogen affect the enantioselectivity of hydrogenation in an opposite way for two enamide reactants, M-acrylate (methyl 2-acetamidoacrylate) and E-emap (ethyl 4-methyl-3-acetamido-2-pentanoate), with rhodium (I) complexes coordinated to a diphosphine ligand? This question was answered by a combination of experiments and DFT calculations. The activation free energies, the...
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