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Vielfalt en gros: Durch palladiumkatalysierte Carbonylierung wird eine hoch regioselektive Triazolsynthese gestartet. Die drei weiteren Partner, Arylhalogenid, Amidin und Hydrazin, lassen sich einfach variieren, was vollständig substituierte 1,2,4‐Triazole in modularer Form zugänglich macht. Das Verfahren wurde zur Synthese wirkstoffartiger und/oder pharmazeutisch wichtiger Moleküle wie Deferasirox...
All 4 one: Palladium‐catalyzed carbonylation initiates a highly regioselective triazole synthesis. In this four‐partner protocol, the aryl halide, amidine, and hydrazine partners are easily varied, allowing the synthesis of fully substituted 1,2,4‐triazoles in a modular fashion. This methodology is demonstrated with the synthesis of druglike and/or pharmaceutically relevant molecules such as deferasirox.
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