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We synthesized a cyanido‐bridged Mn−Nb metal assembly possessing large‐sized bridging ligands with disulfide bonds, [Mn(dpds)2]2[Nb(CN)8] ⋅ 6H2O (MnNb, dpds: 4,4’‐dipyridyldisulfide). MnNb has a three‐dimensional coordination framework in which the Mn and Nb sites are bridged by cyanides, while the Mn sites are combined by dpds ligands. The two crystallographically independent dpds ligands are bent...
This article deals with novel opto-magnetic and magneto-optical phenomena. These phenomena are demonstrated with metal polycyanides, which are classified as molecule-based magnets. Cobalt hexacyanoferrate and copper octacyanomolybdate solids exhibit a photo-reversible enhancement of magnetization. These photo-magnetic phenomena are based on the photo-induced electron transfer between diamagnetic (or...
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