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Two donor‐π‐acceptor (D‐π‐A) dyes are synthesized for application in dye‐sensitized solar cells (DSSC). These D‐π‐A sensitizers use triphenylamine as donor, oligothiophene as both donor and π‐bridge, and benzothiadiazole (BTDA)/cyanoacrylic acid as acceptor that can be anchored to the TiO2 surface. Tuning of the optical and electrochemical properties is observed by the insertion of a phenyl ring between...
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