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Multinuclear heterometallic nanoclusters with controllable stoichiometry and structure are anticipated to possess promising catalytic, magnetic, and optical properties. Heterometallic nanoclusters with precise stoichiometry of Bi3Cu4 and Bi7Cu12 can be stabilized in the scaffold of two‐dimensional metal–organic networks on a Cu(111) surface through on‐surface metallosupramolecular self‐assembly processes...
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