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The melting behavior of a coordination polymer (CP) crystal was utilized to achieve enhanced and optically switchable proton conductivity in the solid state. The strong acid molecules (triflic acid) were doped in one‐dimensional (1D) CP, [Zn(HPO4)(H2PO4)2](ImH2)2 (ImH2=monoprotonated imidazole) in the melt state, and overall enhancement in the proton conductivity was obtained. The enhanced proton...
The glassy state of a two‐dimensional (2D) Cd2+ coordination polymer crystal was prepared by a solvent‐free mechanical milling process. The glassy state retains the 2D structure of the crystalline material, albeit with significant distortion, as characterized by synchrotron X‐ray analyses and solid‐state multinuclear NMR spectroscopy. It transforms to its original crystal structure upon heating. Thus,...
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