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We performed electron spin resonance (ESR) studies of the mixed valence Prussian blue analogue, Rb 0.8 Mn 1.1 [Fe(CN) 6 ]·D 2 O in a wide frequency (9.5–319GHz) and temperature (3.5–300K) interval. Evidence for the proposed high-temperature Mn 2+ (S=52)–NC–Fe 3+ (S=12) to low-temperature Mn 3+ (S=2)–NC–Fe 2+ (S=0) internal charge transfer...
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