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Binuclear alkyne manganese carbonyls of the type (RC≡CR')Mn2(CO)n (R and R'=methyl or dimethylamino; n=8, 7, 6) and their isomers related to the experimentally known (MeC2NEt2)Mn2(CO)n (n=8, 7) structures have been investigated by density functional theory. The alkyne ligand remains intact in the only low energy (Me2N)2C2Mn2(CO)8 isomer, which has a central Mn2C2 tetrahedrane unit and is otherwise...
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