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The peptide‐based porous 3D framework, ZnCar, has been synthesized from Zn2+ and the natural dipeptide carnosine (β‐alanyl‐L‐histidine). Unlike previous extended peptide networks, the imidazole side chain of the histidine residue is deprotonated to afford Zn–imidazolate chains, with bonding similar to the zeolitic imidazolate framework (ZIF) family of porous materials. ZnCar exhibits permanent microporosity...
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