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This manuscript summarizes our recent research results on heterogeneously catalyzed aerobic oxidation reactions using supported metal hydroxide catalysts. Metal hydroxide species possess both Lewis acid and Brønsted base sites on the same metal sites, and various kinds of substrates including alcohols, primary amines, nitriles, and terminal alkynes can be activated by the concerted action of the Lewis...
This article summarizes our recent developments for H2O2- and O2-based green oxidation reactions by polyoxometalates (POMs) and related compounds. POM-based structurally controlled molecular catalysts exhibit high catalytic performance for epoxidation and sulfoxidation with H2O2. These molecular catalysts can be immobilized on the organic–inorganic hybrid support with covalently anchoring N-octyldihydroimidazolium...
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