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Cluster‐based clathrate: Mo4Si4Cla12 inorganic building blocks (see picture, i=inner, a=apical) containing Mo4 metal atom clusters assemble to yield an inorganic giant framework structurally related to type II clathrate. This compound is the first member of a promising family of materials with a wide range of physical properties that combine the chemistry of metallic clusters characterized by delocalized...
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