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The 2014 synthesis of the remarkable dimagnesium compound Mg2[C4(CH3)2(Si(CH3)3)2](C3H7)2(C4H8O)2 may point the way to a new chapter in alkaline earth organometallic chemistry. Accordingly, we have studied the known Mg compound and the analogous Be, Ca, Sr, and Ba structures. Although most of our theoretical predictions come from density functional methods, the latter have been benchmarked using coupled...
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