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Hole or electron doping of phases prepared by topochemical reactions (e.g. anion deintercalation or anion‐exchange) is extremely challenging as these low‐temperature conversion reactions are typically very sensitive to the electron counts of precursor phases. Herein we report the successful hole and electron doping of the transition‐metal oxyhydride LaSr3NiRuO4H4 by first preparing precursors in the...
A series of strontium vanadium oxide–hydride phases prepared by utilizing a low‐temperature synthesis strategy in which oxide ions in Srn+1VnO3n+1 (n=∞, 1, 2) phases are topochemically replaced by hydride ions to form SrVO2H, Sr2VO3H, and Sr3V2O5H2, respectively. These new phases contain sheets or chains of apex‐linked V3+O4 squares stacked with SrH layers/chains, such that the n=∞ member, SrVO2H,...
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