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Two solution‐processable metallopolyynes of platinum functionalized with the electron‐deficient 4H‐cyclopenta[2,1‐b:3,4‐b']dithiophen‐4‐one spacer and their model molecular complexes were synthesized and developed for the applications of polymer solar cells. These metallated polymers possess extremely low bandgaps of 1.44–1.53 eV which extend toward the near‐infrared (NIR) range of the solar spectrum,...
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