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A novel series of aroyl-pyrrolyl-hydroxy-amides (APHAs) active as histone deacetylase (HDAC) inhibitors has been reported. The new derivatives were designed by replacing the benzene ring of the prototype 1 with both aromatic and aliphatic, monocyclic and polycyclic rings (compounds 3a–i), or by inserting a number of substituents on the methylene linker of 1 (compounds 4a–l). Compounds 3a–i and 4a–l...
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