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The theoretical capacity of pristine silicon as anodes for lithium‐ion batteries (LIBs) can reach up to 4200 mAh g−1, however, the low electrical conductivity and the huge volume expansion limit their practical application. To address this challenge, a precursor strategy has been explored to induce the curling of graphene oxide (GO) flakes and the enclosing of Si nanoparticles by selecting protonated...