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Chiral metal‐organic frameworks have shown great potential in enantioselective separation and asymmetric catalysis due to their diverse and adjustable structures with abundant chiral recognition sites. Herein, a new chiral post‐synthetic modification was used for preparing an achiral@chiral metal‐organic frameworks core‐shell composite [Cu3(Btc)2]@[Cu2((+)‐Cam)2Dabco] by a superficial chiral etching...
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