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Hexameric and tetrameric methyllithium were allowed to react with carbon monoxide (or isonitrile) to form a main group metal carbonyl in the first reaction step. The species rearranges to a lithium acetyl via formal insertion of CO into the lithium carbon bond. In a further step it is seen that a substituted ethane is formed, probably via the formation of an oxycarbene intermediate. The results of...
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