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Several new non–symmetrically p–nitrobenzyl substituted benzimidazole–based mono–N–heterocyclic carbene (NHC)–silver(I) acetate (7a–e) and bis–NHC–silver(I) hexafluorophosphate complexes (8a–e) were synthesized by combination of 1–ethyl/1–propyl/1–butyl/1–pentyl/1–hexyl–3–(4–nitrobenzyl)benzimidazolium hexafluorophosphate salts (6a–e) with silver(I) acetate and silver(I) oxide in methanol and acetonitrile,...
From the reaction of 1H‐imidazole (1a), 4,5‐dichloro‐1H‐imidazole (1b), 1H‐benzimidazole (1c), 1‐methyl‐1H‐imidazole (1d), and 1‐methyl‐1H‐benzimidazole (1f) with methyl 4‐(bromomethyl)benzoate (2), symmetrically and nonsymmetrically 4‐(methoxycarbonyl)benzyl‐substituted N‐heterocyclic carbene (NHC) precursors, 3a–3f, were synthesized. These NHC precursors were then reacted with silver(I) acetate...
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