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Unique layered and heterostructured Pd/PdWCr nanosheet‐assembled flowers (L‐Pd/PdWCr) are successfully synthesized, resulting in the most negative onset potential (up to −0.174 V vs SCE) for formic acid oxidation among all reported Pd‐based electrocatalysts. It has 4.3‐times higher catalytic peak current density and better stability than that of the commercial Pd/C. The catalytic enhancement mechanism...
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