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Optical properties and interface energetics between semiconductor and electrolyte determine sensitively the efficiency of a photoelectrode for solar water splitting. By careful design of the involved interfaces and photon management, a record 15.8% power‐saved efficiency single junction InP‐based photoelectrode for photoelectrochemical water reduction can be obtained, as shown on page 679 by L. Gao,...
The solar energy conversion efficiency of photoelectrochemical (PEC) devices is usually limited by poor interface energetics, limiting the onset potential, and light reflection losses. Here, a three‐pronged approach to obtain excellent performance of an InP‐based photoelectrode for water reduction is presented. First, a buried p–n+ junction is fabricated, which shifts the valence band edge favorably...
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