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We report a synthetic approach towards metal complexes of the poorly coordinating sulfonamide 2‐tosylaminomethylaniline (HLTs) that exploits both the good donor capacity of imine N atoms and the hydrolysis of imine ligands mediated by d‐block metals. Zn2+, Cd2+ and Pd2+ ions appear to promote the efficient hydrolysis of a coordinated imine ligand (H2LSB) at room temperature, especially in a protic...
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