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Compared to crown ethers with functions to capture metal cation, inverse crown ethers (ICEs) with a similar cavity architecture have the alternating polarity of cationic metal ring and encapsulated ion to construct the skeleton. Here we introduce a new tridentate aryloxide‐N‐heterocyclic carbene ligand to stabilize μ4‐oxo [Mg4O] cores in ICEs, which open up a path towards synthetic methodology for...
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