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Extensive potential energy surface explorations of twenty‐five clusters with the formula E3M3+ (E=Group 14 element and M=Group 1 element) through density functional theory and high‐level ab initio computations reveal that the lowest‐energy isomer for all these systems corresponds to a non‐classical D3h star‐like structure in the singlet state, where three M atoms interact electrostatically with the...
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