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A series of conjugated polymers comprising polythiophene, polyselenophene, and polytellurophene with branched 3,7‐dimethyloctyl side chains, well‐matched molecular weight, dispersity, and regioregularity is synthesized. The ionization potential is found to vary from 5.14 to 5.32 eV, with polytellurophene having the lowest potential. Field‐effect transistors based on these materials exhibit distinct...
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