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The construction of interlocked topologies by metal‐cation‐template methods has been extensively explored. However, construction of these species using template‐free chemical self‐assembly methods is hard to rationally achieve due to the inherent unpredictability of self‐assembly processes. In this work, a strategy to construct interlocked [2]catenanes by coordination‐driven template‐free self‐assembly...
Herein, we report an artificially assembled interlocked system that features adaptive self‐assembly and induced‐fit transformation properties in the presence of appropriate guest molecules. By careful choice of solvent and guests, a molecular Borromean rings complex based on organometallic half‐sandwich units could be transformed in a stepwise manner to a ring‐in‐ring complex and a monomeric rectangle,...
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