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Based on that the evolution of renewable H2 by using a photochemical method requires photoinduced electron transfer (ET) from a light harvester to an electrocatalyst in water, we present a nickel complex, [BzPyN(CH3)2]2[Ni(i-mnt)2] 1 (i-mnt2−=2,2-dicyanoethylene-1,1-dithiolate) that acts as both an electrocatalyst and a photocatalyst for H2 generation from water via an unstable nickel hydride intermediate...
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