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Lithium batteries occupy the large‐scale electric mobility market raising concerns about the environmental impact of cell production, especially regarding the use of poly(vinylidene difluoride) (teratogenic) and N‐methyl‐2‐pyrrolidone (NMP, harmful). To avoid their use, an aqueous electrode processing route is utilized in which a water‐soluble hybrid acrylic‐fluoropolymer together with sodium carboxymethyl...
Halide‐free, water‐in‐salt electrolytes (WiSEs) composed of potassium acetate (KAc) and zinc acetate (ZnAc2) are investigated as electrolytes in zinc‐ion hybrid supercapacitors (ZHSs). Molecular dynamics simulations demonstrate that water molecules are mostly non‐interacting with each other in the highly concentrated WiSEs, while “bulk‐like water” regions are present in the dilute electrolyte. Among...
In article number 2000279, Maximilian Fichtner, Stefano Passerini, and co‐workers demonstrate improved interfacial properties of a lithium lanthanium zirconate (LLZO) solid‐electrolyte (SE)‐based solid‐state battery by employing ionic liquid interlayers at the electrode/electrolyte junctions. This strategy lowers the interfacial resistances and suppresses Li dendrite formation, thus enabling high...
Li‐garnets are promising inorganic ceramic solid electrolytes for lithium metal batteries, showing good electrochemical stability with Li anode. However, their brittle and stiff nature restricts their intimate contact with both the electrodes, hence presenting high interfacial resistance to the ionic mobility. To address this issue, a strategy employing ionic liquid electrolyte (ILE) thin interlayers...
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