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The effect of CaO on N2O decomposition and the selectivity of its decomposition products (NO and N2) was investigated using a fixed-bed flow reactor with varying temperatures from 317°C to 947°C. The selectivity of NO from CaO-catalyzed N2O decomposition is much lower than the N2 selectivity with the N2/NO products ratio greater than 12.1. Compared to N2O homogeneous decomposition with the minimum...
The catalytic effect of CaS on N2O decomposition and reduction was investigated using density functional theory calculations. N2O approached the CaS (100) surface and crossed an energy barrier of 1.228eV, decomposing into a free N2 molecule and an adsorbed O atom. The generated adsorbed O atom could be removed through two reaction pathways: binding with a neighboring adsorbed O atom into O2 with the...
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